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irradiation for 10 min, and TEM image of the colloids before light irradiation is also given for comparison. It can be seen that after the irradiation, the spheres are deformed to ellipsoids, which can also be con rmed by AFM observations. The elongation occurs in the polarization direction of the laser beam, which is also the grating vector direction of the interference patterns. In the testing period (15 min), the colloids can be continuously elongated by the light irradiation. The average major-to-minor axis ratio (l/d) of the colloids can be used to indicate the deformation degree of the colloids. Figure 5.11 shows the SEM images of colloidal particles observed before the irradiation and after the irradiation for different time periods. After 5-min irradiation, obvious change in the shape can be observed. As the irradiation time increases, the elongation can be observed to increase continuously. The relationship between the average major-tominor ratio (estimated statistically from SEM images of 100 colloidal particles) and the irradiation time is given in Fig. 5.12. The major-to-minor ratio increases almost linearly with the irradiation time increase in the testing range. The colloidal sphere deformation could be attributed to the optically induced electric eld gradient, which has been used by Kumar et al. (1998) to explain the SRG formation. The polymers used to construct the photodeformable colloids can also show sensitive properties to form SRG. Photoinduced mass migration has been used to account for the SRG formation, where the polymer chains are driven by light to move from bright to dark regions. The colloid deformation could also be caused by the mass migration related to the electric eld gradient force. download barcode macro for excel Barcode in Excel
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